LAPSE:2024.0268
Postprint
LAPSE:2024.0268
The design and operational space of syngas production via integrated direct air capture with gaseous CO2 electrolysis
April 4, 2024
The overarching goal of limiting the increase in global temperature to ≤ 2.0˚ C likely requires both decarbonization and defossilization efforts. Direct air capture (DAC) and CO2 electrolysis stand out as promising technologies for capturing and utilizing atmospheric CO2. In this effort, we explore the details of designing and operating an integrated DAC-electrolysis process by examining some key parameters for economic feasibility. We evaluate the gross profit and net income to find the most appropriate capacity factor, average electricity price, syngas sale price, and CO2 taxes. Additionally, we study an optimistic scenario of CO2 electrolysis and perform a sensitivity analysis of the CO2 capture price to elucidate the impact of design decisions on the economic feasibility. Our findings underscore the necessity of design improvements of the CO2 electrolysis and DAC processes to achieve reasonable capacity factor and average electricity price limits. Notably, CO2 taxes and tax credits in the order of $400 per t-CO2 or greater are essential for the economic viability of the optimistic DAC-electrolysis route, especially at competitive syngas sale prices. This study serves as a foundation for further work on designing appropriate power system models that integrate well with the presented air-to-syngas route.
Keywords
Carbon Dioxide Capture, CO2 electrolysis, Direct air capture, Modelling, Syngas, Technoeconomic Analysis
Suggested Citation
Almajed HM, Guerra OJ, Somoza-Tornos A, Smith WA, Hodge BM. The design and operational space of syngas production via integrated direct air capture with gaseous CO2 electrolysis. (2024). LAPSE:2024.0268
Author Affiliations
Almajed HM: University of Colorado Boulder [ORCID] [Google Scholar]
Guerra OJ: National Renewable Energy Laboratory [ORCID]
Somoza-Tornos A: TU Delft [ORCID] [Google Scholar]
Smith WA: University of Colorado Boulder; National Renewable Energy Laboratory [ORCID] [Google Scholar]
Hodge BM: University of Colorado Boulder; National Renewable Energy Laboratory [ORCID] [Google Scholar]
[Login] to see author email addresses.
Journal Name
Systems & Control Transactions
Year
2024
Version Comments
Original Submission
Record Map
External Link

doi:10.1039/D3EE02589F
Predecessor work
Postprint

LAPSE:2024.0268
This Record
Download
Files
[Download 1v1.pdf] (970 kB)
Apr 4, 2024
Supplementary Information
License
None Specified
 
Meta
Record Statistics
Record Views
47
Version History
[v1] (Original Submission)
Apr 4, 2024
 
Verified by curator on
Apr 11, 2024
This Version Number
v1
Citations
Most Recent
This Version
URL Here
https://psecommunity.org/LAPSE:2024.0268
 
Original Submitter
hual7301
Links to Related Works
Predecessor Works
Predecessor work