Grinding is widely used in mechanical manufacturing to obtain both precision and part requirements. In order to achieve carbon efficiency improvement and save costs, carbon emission and processing cost models of the grinding process are established in this study. In the modeling process, a speed-change-based adjustment function was introduced to dynamically derive the change of the target model. The carbon emission model was derived from the grinding force using regression. Considering the constraints of machine tool equipment performance and processing quality requirements, the grinding wheel’s linear velocity, cutting feed rate, and the rotation speed of the workpiece were selected as the optimization variables, and the improved NSGA-II algorithm was applied to solve the optimization model. Finally, fuzzy matter element analysis was used to evaluate the most optimal processing plan.