LAPSE:2023.6147v1
Published Article

LAPSE:2023.6147v1
Numerical Simulation on Effect of Separator Thickness on Coupling Phenomena in Single Cell of PEFC under Higher Temperature Operation Condition at 363 K and 373 K
February 23, 2023
Abstract
In hydrogen energy systems, the polymer electrolyte fuel cell (PEFC) is an important component. The purpose of this study is to clarify the effect of separator thickness (s.t.) in PEFC on the distributions of mass such as H2, O2, H2O and current density when PEFC is operated at 363 K and 373 K. The relative humidity (RH) of supply gases also impacts the operation. The numerical simulation (using a 3D model) with COMSOL Multiphysics has been conducted to analyze the characteristics of PEFC. It has been observed that the molar concentration of H2 using s.t. of 2.0 mm is smaller compared with the thinner s.t. cases at the initial operation temperature of a cell (Tini) = 363 K and 373 K. The molar concentration of O2 using s.t. of 2.0 mm is smaller compared with the thinner s.t. cases at Tini = 373 K, as well as the case for the RH of supply gases at the anode of 40%RH and cathode of 40%RH (A40%RH/C40%RH) irrespective of Tini. Additionally, it has been clarified that the molar concentration of H2O maintains a low value along with the gas channel at Tini = 373 K using s.t. of 1.5 mm and 1.0 mm. Moreover, it has been clarified that the current density using s.t. of 2.0 mm is the highest among the different s.t. irrespective of Tini, which is the most remarkable in the case of A40%RH&C40%RH.
In hydrogen energy systems, the polymer electrolyte fuel cell (PEFC) is an important component. The purpose of this study is to clarify the effect of separator thickness (s.t.) in PEFC on the distributions of mass such as H2, O2, H2O and current density when PEFC is operated at 363 K and 373 K. The relative humidity (RH) of supply gases also impacts the operation. The numerical simulation (using a 3D model) with COMSOL Multiphysics has been conducted to analyze the characteristics of PEFC. It has been observed that the molar concentration of H2 using s.t. of 2.0 mm is smaller compared with the thinner s.t. cases at the initial operation temperature of a cell (Tini) = 363 K and 373 K. The molar concentration of O2 using s.t. of 2.0 mm is smaller compared with the thinner s.t. cases at Tini = 373 K, as well as the case for the RH of supply gases at the anode of 40%RH and cathode of 40%RH (A40%RH/C40%RH) irrespective of Tini. Additionally, it has been clarified that the molar concentration of H2O maintains a low value along with the gas channel at Tini = 373 K using s.t. of 1.5 mm and 1.0 mm. Moreover, it has been clarified that the current density using s.t. of 2.0 mm is the highest among the different s.t. irrespective of Tini, which is the most remarkable in the case of A40%RH&C40%RH.
Record ID
Keywords
higher temperature, mass and current density distribution, numerical simulation, PEFC, relative humidity, separator thickness
Subject
Suggested Citation
Nishimura A, Mishima D, Toyoda K, Ito S, Kolhe ML. Numerical Simulation on Effect of Separator Thickness on Coupling Phenomena in Single Cell of PEFC under Higher Temperature Operation Condition at 363 K and 373 K. (2023). LAPSE:2023.6147v1
Author Affiliations
Nishimura A: Division of Mechanical Engineering, Graduate School of Engineering, Mie University, 1577 Kurimamachiya-cho, Tsu 514-8507, Japan [ORCID]
Mishima D: Division of Mechanical Engineering, Graduate School of Engineering, Mie University, 1577 Kurimamachiya-cho, Tsu 514-8507, Japan
Toyoda K: Division of Mechanical Engineering, Graduate School of Engineering, Mie University, 1577 Kurimamachiya-cho, Tsu 514-8507, Japan
Ito S: Division of Mechanical Engineering, Graduate School of Engineering, Mie University, 1577 Kurimamachiya-cho, Tsu 514-8507, Japan
Kolhe ML: Faculty of Engineering and Science, University of Agder, P.O. Box 422, NO-4604 Kristiansand, Norway [ORCID]
Mishima D: Division of Mechanical Engineering, Graduate School of Engineering, Mie University, 1577 Kurimamachiya-cho, Tsu 514-8507, Japan
Toyoda K: Division of Mechanical Engineering, Graduate School of Engineering, Mie University, 1577 Kurimamachiya-cho, Tsu 514-8507, Japan
Ito S: Division of Mechanical Engineering, Graduate School of Engineering, Mie University, 1577 Kurimamachiya-cho, Tsu 514-8507, Japan
Kolhe ML: Faculty of Engineering and Science, University of Agder, P.O. Box 422, NO-4604 Kristiansand, Norway [ORCID]
Journal Name
Energies
Volume
16
Issue
2
First Page
606
Year
2023
Publication Date
2023-01-04
ISSN
1996-1073
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Original Submission
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PII: en16020606, Publication Type: Journal Article
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LAPSE:2023.6147v1
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