LAPSE:2023.31200
Published Article
LAPSE:2023.31200
A Mini Review: Recent Advances in Asymmetrically Coordinated Atom Sites for High-Efficiency Hydrogen Evolution Reaction
April 18, 2023
Abstract
Energy is the substance foundation of human society. Single−atom catalysts (SACs) have emerged as promising electrode materials in the energy field owing to their unique characteristics. It was demonstrated that the hydrogen evolution reaction (HER) performance of SACs relies on the metal−centric species and the corresponding local coordination engineering. Herein, the recent progress relating to asymmetric atomic catalysts for the HER is reviewed, including low coordination, heteroatomic coordination, and bimetallic coordination. In addition, the connection between the coordination structures and the presented electrocatalytic performance was discussed. The main challenges that need to be addressed for the asymmetric atomic catalysts in the HER are summarized. Finally, some insights into the development of high−quality asymmetric atomic catalysts are included.
Energy is the substance foundation of human society. Single−atom catalysts (SACs) have emerged as promising electrode materials in the energy field owing to their unique characteristics. It was demonstrated that the hydrogen evolution reaction (HER) performance of SACs relies on the metal−centric species and the corresponding local coordination engineering. Herein, the recent progress relating to asymmetric atomic catalysts for the HER is reviewed, including low coordination, heteroatomic coordination, and bimetallic coordination. In addition, the connection between the coordination structures and the presented electrocatalytic performance was discussed. The main challenges that need to be addressed for the asymmetric atomic catalysts in the HER are summarized. Finally, some insights into the development of high−quality asymmetric atomic catalysts are included.
Record ID
Keywords
asymmetric atom sites, catalyst design, coordination environment, hydrogen evolution reaction
Subject
Suggested Citation
Ding J, Liu W, Zhang S, Luo J, Liu X. A Mini Review: Recent Advances in Asymmetrically Coordinated Atom Sites for High-Efficiency Hydrogen Evolution Reaction. (2023). LAPSE:2023.31200
Author Affiliations
Ding J: Institute for New Energy Materials and Low-Carbon Technologies, School of Materials Science and Engineering, Tianjin University of Technology, Tianjin 300384, China; State Key Laboratory of Featured Metal Materials and Life-Cycle Safety for Composite Stru
Liu W: College of Materials Science and Engineering, Zhejiang University of Technology, 18 Chaowang Road, Hangzhou 310014, China
Zhang S: College of Chemistry, Zhengzhou University, Zhengzhou 450001, China
Luo J: Institute for New Energy Materials and Low-Carbon Technologies, School of Materials Science and Engineering, Tianjin University of Technology, Tianjin 300384, China; Shensi Laboratory, Shenzhen Institute for Advanced Study, University of Electronic Scienc
Liu X: State Key Laboratory of Featured Metal Materials and Life-Cycle Safety for Composite Structures, School of Resource, Environments and Materials, Nanning 530004, China [ORCID]
Liu W: College of Materials Science and Engineering, Zhejiang University of Technology, 18 Chaowang Road, Hangzhou 310014, China
Zhang S: College of Chemistry, Zhengzhou University, Zhengzhou 450001, China
Luo J: Institute for New Energy Materials and Low-Carbon Technologies, School of Materials Science and Engineering, Tianjin University of Technology, Tianjin 300384, China; Shensi Laboratory, Shenzhen Institute for Advanced Study, University of Electronic Scienc
Liu X: State Key Laboratory of Featured Metal Materials and Life-Cycle Safety for Composite Structures, School of Resource, Environments and Materials, Nanning 530004, China [ORCID]
Journal Name
Energies
Volume
16
Issue
6
First Page
2664
Year
2023
Publication Date
2023-03-12
ISSN
1996-1073
Version Comments
Original Submission
Other Meta
PII: en16062664, Publication Type: Review
Record Map
Published Article
LAPSE:2023.31200
This Record
External Link
https://doi.org/10.3390/en16062664
Publisher Version
Download
Meta
Record Statistics
Record Views
157
Version History
[v1] (Original Submission)
Apr 18, 2023
Verified by curator on
Apr 18, 2023
This Version Number
v1
Citations
Most Recent
This Version
URL Here
https://psecommunity.org/LAPSE:2023.31200
Record Owner
Auto Uploader for LAPSE
Links to Related Works