LAPSE:2023.1964v1
Published Article
LAPSE:2023.1964v1
Model-Based Investigation of the Interaction of Gas-Consuming Reactions and Internal Circulation Flow within Jet Loop Reactors
February 21, 2023
Abstract
Jet loop reactors are standard multiphase reactors used in chemical, biological and environmental processes. The strong liquid jet provided by a nozzle enforces both internal circulation of liquid and gas as well as entrainment and dispersion of the gas phase. We present a one-dimensional compartment model based on a momentum balance that describes the internal circulation of gas and liquid phase in the jet loop reactor. This model considers the influence of local variations of the gas volume fraction on the internal circulation. These local variations can be caused by coalescence of gas bubbles, additional gas-feeding points and gas consumption or production. In this work, we applied the model to study the influence of a gas-consuming reaction on the internal circulation. In a comprehensive sensitivity analysis, the interaction of different parameters such as rate of reaction, power input through the nozzle, gas holdup, reactor geometry, and circulation rate were investigated. The results show that gas consumption can have a significant impact on internal circulation. Industrially relevant operating conditions have even been found where the internal circulation comes to a complete standstill.
Keywords
compartment model, jet loop reactor, multifluid, one-dimensional model, reactive multiphase flow, sensitivity analysis, stability
Suggested Citation
Breit F, Bey O, von Harbou E. Model-Based Investigation of the Interaction of Gas-Consuming Reactions and Internal Circulation Flow within Jet Loop Reactors. (2023). LAPSE:2023.1964v1
Author Affiliations
Breit F: Laboratory of Reaction and Fluid Process Engineering, Technische Universität Kaiserslautern, Gottlieb-Daimler-Straße 44, 67663 Kaiserslautern, Germany [ORCID]
Bey O: Process Research & Chemical Engineering, BASF SE, Carl-Bosch-Str. 38, 67056 Ludwigshafen, Germany
von Harbou E: Laboratory of Reaction and Fluid Process Engineering, Technische Universität Kaiserslautern, Gottlieb-Daimler-Straße 44, 67663 Kaiserslautern, Germany [ORCID]
Journal Name
Processes
Volume
10
Issue
7
First Page
1297
Year
2022
Publication Date
2022-06-30
ISSN
2227-9717
Version Comments
Original Submission
Other Meta
PII: pr10071297, Publication Type: Journal Article
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LAPSE:2023.1964v1
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https://doi.org/10.3390/pr10071297
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Feb 21, 2023
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