LAPSE:2023.1038
Published Article

LAPSE:2023.1038
3D Printing Multi-Channel Large Volume Microchannel Reactor for Enhanced Removal of Low-Concentration NOx Flue Gas
February 21, 2023
Abstract
Compared with conventional reactors that are designed by traditional micromachining technology, the use of 3D-printing technology to manufacture multichannel large-volume microchannel reactors as reaction equipment to remove low-concentration NOX by the wet method is simple and convenient, and the processing cost is low. The results showed that when the concentration of NO was 400 ppm, the mixed solution of (NH2)2CO mass fraction of 3% and H2O2 concentration of 0.5 mol/L was used, and the flow rates of gas and liquid were 100 mL/min, respectively, under the experimental conditions of pH = 11, solution temperature of 20 °C and 500 mL solution recycling for 20 min, the best removal effect of NOX was achieved, and the removal efficiency was 100%. When the O2 content in the flue gas was increased and the number and length of microchannels were increased, the NOX removal efficiency increased accordingly, which was conducive to the rapid and efficient reaction. The application of the microchannel reactor presents a new method for improving the air quality and reducing environmental pollution in the future.
Compared with conventional reactors that are designed by traditional micromachining technology, the use of 3D-printing technology to manufacture multichannel large-volume microchannel reactors as reaction equipment to remove low-concentration NOX by the wet method is simple and convenient, and the processing cost is low. The results showed that when the concentration of NO was 400 ppm, the mixed solution of (NH2)2CO mass fraction of 3% and H2O2 concentration of 0.5 mol/L was used, and the flow rates of gas and liquid were 100 mL/min, respectively, under the experimental conditions of pH = 11, solution temperature of 20 °C and 500 mL solution recycling for 20 min, the best removal effect of NOX was achieved, and the removal efficiency was 100%. When the O2 content in the flue gas was increased and the number and length of microchannels were increased, the NOX removal efficiency increased accordingly, which was conducive to the rapid and efficient reaction. The application of the microchannel reactor presents a new method for improving the air quality and reducing environmental pollution in the future.
Record ID
Keywords
3D printing, H2O2, microchannel reactor, NOX, urea
Subject
Suggested Citation
Han K, Ju S, Zhou Y, Zhang J, Wan X, Li N, Gu Y. 3D Printing Multi-Channel Large Volume Microchannel Reactor for Enhanced Removal of Low-Concentration NOx Flue Gas. (2023). LAPSE:2023.1038
Author Affiliations
Han K: Faculty of Metallurgical and Energy Engineering, Kunming University of Science and Technology, Kunming 650093, China; State Key Laboratory of Complex Nonferrous Metal Resources Clean Utilization, Kunming University of Science and Technology, Kunming 65009
Ju S: Faculty of Metallurgical and Energy Engineering, Kunming University of Science and Technology, Kunming 650093, China; State Key Laboratory of Complex Nonferrous Metal Resources Clean Utilization, Kunming University of Science and Technology, Kunming 65009
Zhou Y: Faculty of Metallurgical and Energy Engineering, Kunming University of Science and Technology, Kunming 650093, China; State Key Laboratory of Complex Nonferrous Metal Resources Clean Utilization, Kunming University of Science and Technology, Kunming 65009
Zhang J: Faculty of Metallurgical and Energy Engineering, Kunming University of Science and Technology, Kunming 650093, China; State Key Laboratory of Complex Nonferrous Metal Resources Clean Utilization, Kunming University of Science and Technology, Kunming 65009
Wan X: Faculty of Metallurgical and Energy Engineering, Kunming University of Science and Technology, Kunming 650093, China; State Key Laboratory of Complex Nonferrous Metal Resources Clean Utilization, Kunming University of Science and Technology, Kunming 65009
Li N: Faculty of Metallurgical and Energy Engineering, Kunming University of Science and Technology, Kunming 650093, China; State Key Laboratory of Complex Nonferrous Metal Resources Clean Utilization, Kunming University of Science and Technology, Kunming 65009
Gu Y: Kunming Institute of Precious Metals, Kunming 650106, China
Ju S: Faculty of Metallurgical and Energy Engineering, Kunming University of Science and Technology, Kunming 650093, China; State Key Laboratory of Complex Nonferrous Metal Resources Clean Utilization, Kunming University of Science and Technology, Kunming 65009
Zhou Y: Faculty of Metallurgical and Energy Engineering, Kunming University of Science and Technology, Kunming 650093, China; State Key Laboratory of Complex Nonferrous Metal Resources Clean Utilization, Kunming University of Science and Technology, Kunming 65009
Zhang J: Faculty of Metallurgical and Energy Engineering, Kunming University of Science and Technology, Kunming 650093, China; State Key Laboratory of Complex Nonferrous Metal Resources Clean Utilization, Kunming University of Science and Technology, Kunming 65009
Wan X: Faculty of Metallurgical and Energy Engineering, Kunming University of Science and Technology, Kunming 650093, China; State Key Laboratory of Complex Nonferrous Metal Resources Clean Utilization, Kunming University of Science and Technology, Kunming 65009
Li N: Faculty of Metallurgical and Energy Engineering, Kunming University of Science and Technology, Kunming 650093, China; State Key Laboratory of Complex Nonferrous Metal Resources Clean Utilization, Kunming University of Science and Technology, Kunming 65009
Gu Y: Kunming Institute of Precious Metals, Kunming 650106, China
Journal Name
Processes
Volume
11
Issue
1
First Page
158
Year
2023
Publication Date
2023-01-04
ISSN
2227-9717
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PII: pr11010158, Publication Type: Journal Article
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LAPSE:2023.1038
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https://doi.org/10.3390/pr11010158
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