LAPSE:2023.28911
Published Article

LAPSE:2023.28911
CO2 Convective Dissolution in Oil-Saturated Unconsolidated Porous Media at Reservoir Conditions
April 12, 2023
Abstract
During CO2 storage, CO2 plume mixes with the water and oil present at the reservoir, initiated by diffusion followed by a density gradient that leads to a convective flow. Studies are available where CO2 convective mixing have been studied in water phase but limited in oil phase. This study was conducted to reach this gap, and experiments were conducted in a vertically packed 3-dimensional column with oil-saturated unconsolidated porous media at 100 bar and 50 °C (representative of reservoir pressure and temperature conditions). N-Decane and crude oil were used as oils, and glass beads as porous media. A bromothymol blue water solution-filled sapphire cell connected at the bottom of the column was used to monitor the CO2 breakthrough. With the increase of the Rayleigh number, the CO2 transport rate in n-decane was found to increase as a function of a second order polynomial. Ra number vs. dimensionless time τ had a power relationship in the form of Ra = c×τ−n. The overall pressure decay was faster in n-decane compared to crude oil for similar permeability (4 D), and the crude oil had a breakthrough time three times slower than in n-decane. The results were compared with similar experiments that have been carried out using water.
During CO2 storage, CO2 plume mixes with the water and oil present at the reservoir, initiated by diffusion followed by a density gradient that leads to a convective flow. Studies are available where CO2 convective mixing have been studied in water phase but limited in oil phase. This study was conducted to reach this gap, and experiments were conducted in a vertically packed 3-dimensional column with oil-saturated unconsolidated porous media at 100 bar and 50 °C (representative of reservoir pressure and temperature conditions). N-Decane and crude oil were used as oils, and glass beads as porous media. A bromothymol blue water solution-filled sapphire cell connected at the bottom of the column was used to monitor the CO2 breakthrough. With the increase of the Rayleigh number, the CO2 transport rate in n-decane was found to increase as a function of a second order polynomial. Ra number vs. dimensionless time τ had a power relationship in the form of Ra = c×τ−n. The overall pressure decay was faster in n-decane compared to crude oil for similar permeability (4 D), and the crude oil had a breakthrough time three times slower than in n-decane. The results were compared with similar experiments that have been carried out using water.
Record ID
Keywords
3-dimensional column, CO2 dissolution, convection, oil, porous media, reservoir conditions
Subject
Suggested Citation
Amarasinghe W, Fjelde I, Giske N, Guo Y. CO2 Convective Dissolution in Oil-Saturated Unconsolidated Porous Media at Reservoir Conditions. (2023). LAPSE:2023.28911
Author Affiliations
Amarasinghe W: NORCE Norwegian Research Center AS, P.O. Box 8046, 4068 Stavanger, Norway; Department of Energy Resources, University of Stavanger, P.O. Box 8600, 4036 Stavanger, Norway
Fjelde I: NORCE Norwegian Research Center AS, P.O. Box 8046, 4068 Stavanger, Norway [ORCID]
Giske N: NORCE Norwegian Research Center AS, P.O. Box 8046, 4068 Stavanger, Norway
Guo Y: NORCE Norwegian Research Center AS, P.O. Box 8046, 4068 Stavanger, Norway; Department of Energy Resources, University of Stavanger, P.O. Box 8600, 4036 Stavanger, Norway
Fjelde I: NORCE Norwegian Research Center AS, P.O. Box 8046, 4068 Stavanger, Norway [ORCID]
Giske N: NORCE Norwegian Research Center AS, P.O. Box 8046, 4068 Stavanger, Norway
Guo Y: NORCE Norwegian Research Center AS, P.O. Box 8046, 4068 Stavanger, Norway; Department of Energy Resources, University of Stavanger, P.O. Box 8600, 4036 Stavanger, Norway
Journal Name
Energies
Volume
14
Issue
1
Article Number
E233
Year
2021
Publication Date
2021-01-04
ISSN
1996-1073
Version Comments
Original Submission
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PII: en14010233, Publication Type: Journal Article
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LAPSE:2023.28911
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https://doi.org/10.3390/en14010233
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Apr 12, 2023
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