LAPSE:2023.16608v1
Published Article

LAPSE:2023.16608v1
Planar Laser-Induced Fluorescence and Chemiluminescence Analyses of CO2-Argon-Steam Oxyfuel (CARSOXY) Combustion
March 3, 2023
Abstract
Strict regulations and acts have been imposed to limit NOx and carbon emissions. The power generation industry has resorted to innovative techniques to overcome such a low level of tolerance. Amongst those in the literature, CO2-argon-steam oxyfuel (CARSOXY) gas turbines have theoretically been proven to offer an economically sustainable solution while retaining high efficiency. Although theoretical studies have characterized CARSOXY, no experimental evidence has been provided in the literature. Therefore, this paper attempts to experimentally assess CARSOXY in comparison to a CH4/air flame. OH* chemiluminescence integrated with OH Planar Laser-Induced Fluorescence (PLIF) imaging has been utilized to study flame stability and flame geometry (i.e., the area of highest heat intensity (AOH¯Max center of highest heat intensity (COH¯Max)) over a range of working fluid Reynolds’ numbers and oxidizing equivalence ratios. In addition, the standard deviation of heat release fluctuations (σOH*/OH¯) has been utilized as the base-criteria to compare the stability performance of CARSOXY to CH4/air combustion. Moreover, turbulence-chemistry interactions have been described using Damköhler numbers and by plotting Borghi regime diagrams. This paper suggests a modified numerical approach to estimate Damköhler numbers and plot regime diagrams for non-premixed combustion by utilizing the Buckingham π theorem based on experimental observations and results. CARSOXY flames showed lower flame intensity than that of the CH4/air flame throughout the entire Re interval by approximately 16%, indicating higher heat release. The Damköhler numbers of the CARSOXY flame were also greater than those of the CH4/air flame in all conditions, indicating more uniform CARSOXY flames. It was found that the tendency of the CARSOXY flame of approaching the concentrated reaction zone is greater than that of the CH4/air flame.
Strict regulations and acts have been imposed to limit NOx and carbon emissions. The power generation industry has resorted to innovative techniques to overcome such a low level of tolerance. Amongst those in the literature, CO2-argon-steam oxyfuel (CARSOXY) gas turbines have theoretically been proven to offer an economically sustainable solution while retaining high efficiency. Although theoretical studies have characterized CARSOXY, no experimental evidence has been provided in the literature. Therefore, this paper attempts to experimentally assess CARSOXY in comparison to a CH4/air flame. OH* chemiluminescence integrated with OH Planar Laser-Induced Fluorescence (PLIF) imaging has been utilized to study flame stability and flame geometry (i.e., the area of highest heat intensity (AOH¯Max center of highest heat intensity (COH¯Max)) over a range of working fluid Reynolds’ numbers and oxidizing equivalence ratios. In addition, the standard deviation of heat release fluctuations (σOH*/OH¯) has been utilized as the base-criteria to compare the stability performance of CARSOXY to CH4/air combustion. Moreover, turbulence-chemistry interactions have been described using Damköhler numbers and by plotting Borghi regime diagrams. This paper suggests a modified numerical approach to estimate Damköhler numbers and plot regime diagrams for non-premixed combustion by utilizing the Buckingham π theorem based on experimental observations and results. CARSOXY flames showed lower flame intensity than that of the CH4/air flame throughout the entire Re interval by approximately 16%, indicating higher heat release. The Damköhler numbers of the CARSOXY flame were also greater than those of the CH4/air flame in all conditions, indicating more uniform CARSOXY flames. It was found that the tendency of the CARSOXY flame of approaching the concentrated reaction zone is greater than that of the CH4/air flame.
Record ID
Keywords
Borghi regime diagram, CARSOXY, chemiluminescence, Damköhler number, oxyfuel, PLIF
Subject
Suggested Citation
Fawwaz Alrebei O, I. Amhamed A, Mashruk S, Bowen P, Valera Medina A. Planar Laser-Induced Fluorescence and Chemiluminescence Analyses of CO2-Argon-Steam Oxyfuel (CARSOXY) Combustion. (2023). LAPSE:2023.16608v1
Author Affiliations
Fawwaz Alrebei O: Mechanical and Aerospace Engineering Department, Cardiff School of Engineering, Queen’s Buildings, 14-17 The Parade, Cardiff CF24 3AA, UK; Qatar Environment and Energy Research Institute, Hamad Bin Khalifa University, Doha 5825, Qatar; Aircraft Maintena
I. Amhamed A: Qatar Environment and Energy Research Institute, Hamad Bin Khalifa University, Doha 5825, Qatar [ORCID]
Mashruk S: Mechanical and Aerospace Engineering Department, Cardiff School of Engineering, Queen’s Buildings, 14-17 The Parade, Cardiff CF24 3AA, UK; Gas Turbine Research Centre, Cardiff University, Port Talbot, Cardiff SA13 2EZ, UK [ORCID]
Bowen P: Mechanical and Aerospace Engineering Department, Cardiff School of Engineering, Queen’s Buildings, 14-17 The Parade, Cardiff CF24 3AA, UK; Gas Turbine Research Centre, Cardiff University, Port Talbot, Cardiff SA13 2EZ, UK
Valera Medina A: Mechanical and Aerospace Engineering Department, Cardiff School of Engineering, Queen’s Buildings, 14-17 The Parade, Cardiff CF24 3AA, UK; Gas Turbine Research Centre, Cardiff University, Port Talbot, Cardiff SA13 2EZ, UK [ORCID]
I. Amhamed A: Qatar Environment and Energy Research Institute, Hamad Bin Khalifa University, Doha 5825, Qatar [ORCID]
Mashruk S: Mechanical and Aerospace Engineering Department, Cardiff School of Engineering, Queen’s Buildings, 14-17 The Parade, Cardiff CF24 3AA, UK; Gas Turbine Research Centre, Cardiff University, Port Talbot, Cardiff SA13 2EZ, UK [ORCID]
Bowen P: Mechanical and Aerospace Engineering Department, Cardiff School of Engineering, Queen’s Buildings, 14-17 The Parade, Cardiff CF24 3AA, UK; Gas Turbine Research Centre, Cardiff University, Port Talbot, Cardiff SA13 2EZ, UK
Valera Medina A: Mechanical and Aerospace Engineering Department, Cardiff School of Engineering, Queen’s Buildings, 14-17 The Parade, Cardiff CF24 3AA, UK; Gas Turbine Research Centre, Cardiff University, Port Talbot, Cardiff SA13 2EZ, UK [ORCID]
Journal Name
Energies
Volume
15
Issue
1
First Page
263
Year
2021
Publication Date
2021-12-31
ISSN
1996-1073
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Original Submission
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PII: en15010263, Publication Type: Journal Article
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LAPSE:2023.16608v1
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https://doi.org/10.3390/en15010263
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