From conventional turbines to cutting-edge bladeless turbines, energy harvesting from wind has been well explored by researchers for more than a century. The vortex bladeless wind turbine (VBT) is considered an advanced design that alternatively harvests energy from oscillation. This research investigates enhancing the output electrical power of VBT through simulation of the fluid−solid interactions (FSI), leading to a comprehensive dataset for predicting procedure and optimal design. Hence, the long short-term memory (LSTM) method, due to its time-series prediction accuracy, is proposed to model the power of VBT from the collected data. To find the relationship between the parameters and the variables used in this research, a correlation matrix is further presented. According to the value of 0.3 for the root mean square error (RMSE), a comparative analysis between the simulation results and their predictions indicates that the LSTM method is suitable for modeling. Furthermore, the LSTM method has significantly reduced the computation time so that the prediction time of desired values has been reduced from an average of two and a half hours to two minutes. In addition, one of the most important achievements of this study is to suggest a mathematical relation of output power, which helps to extend it in different sizes of VBT with a high range of parameter variations.