LAPSE:2023.2826
Published Article

LAPSE:2023.2826
Pilot-Scale Experimental Study of a New High-Loading Absorbent for Capturing CO2 from Flue Gas
February 21, 2023
Abstract
Chemical absorbents with low-energy requirements have become the primary focus of the research on CO2 capture from flue gas in power plants. To verify the absorption performance of the NICE absorbent developed by the National Institute of Clean-and-Low-Carbon Energy in China, a performance optimization test was conducted in Zhejiang University’s pilot-scale platform, and the effects of the liquid−gas ratio, regeneration pressure, rich liquid fractional flow, and interstage cooling on the absorption performance and regeneration energy consumption were investigated. The results showed that in the CO2 pilot test, the optimized minimum regeneration energy consumption was 2.85 GJ/t CO2, and the corresponding process parameters were as follows: a liquid−gas ratio of 1.82 L/m3, regeneration pressure of 191 kPa, an interstage cooling temperature of 40 °C, and a rich liquid fractional flow ratio of 0.18. This study preliminarily verified the low-energy consumption performance of the NICE absorbent and showed its good potential for industrial applications. Additionally, the NICE absorbent showed promise for capital and operating cost savings because of its low liquid−gas ratio.
Chemical absorbents with low-energy requirements have become the primary focus of the research on CO2 capture from flue gas in power plants. To verify the absorption performance of the NICE absorbent developed by the National Institute of Clean-and-Low-Carbon Energy in China, a performance optimization test was conducted in Zhejiang University’s pilot-scale platform, and the effects of the liquid−gas ratio, regeneration pressure, rich liquid fractional flow, and interstage cooling on the absorption performance and regeneration energy consumption were investigated. The results showed that in the CO2 pilot test, the optimized minimum regeneration energy consumption was 2.85 GJ/t CO2, and the corresponding process parameters were as follows: a liquid−gas ratio of 1.82 L/m3, regeneration pressure of 191 kPa, an interstage cooling temperature of 40 °C, and a rich liquid fractional flow ratio of 0.18. This study preliminarily verified the low-energy consumption performance of the NICE absorbent and showed its good potential for industrial applications. Additionally, the NICE absorbent showed promise for capital and operating cost savings because of its low liquid−gas ratio.
Record ID
Keywords
absorbent, Carbon Dioxide, NICE, pilot-scale experiment, process optimization, regeneration energy
Subject
Suggested Citation
Ye Y, Zhao X, Chen J, Fang M. Pilot-Scale Experimental Study of a New High-Loading Absorbent for Capturing CO2 from Flue Gas. (2023). LAPSE:2023.2826
Author Affiliations
Ye Y: National Institute of Clean-and-Low-Carbon Energy, Beijing 102211, China
Zhao X: National Institute of Clean-and-Low-Carbon Energy, Beijing 102211, China
Chen J: State Key Laboratory of Chemical Engineering, Tsinghua University, Beijing 100084, China
Fang M: State Key Laboratory of Clean Energy Utilization, Zhejiang University, Hangzhou 310027, China
Zhao X: National Institute of Clean-and-Low-Carbon Energy, Beijing 102211, China
Chen J: State Key Laboratory of Chemical Engineering, Tsinghua University, Beijing 100084, China
Fang M: State Key Laboratory of Clean Energy Utilization, Zhejiang University, Hangzhou 310027, China
Journal Name
Processes
Volume
10
Issue
3
First Page
599
Year
2022
Publication Date
2022-03-19
ISSN
2227-9717
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Original Submission
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PII: pr10030599, Publication Type: Journal Article
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LAPSE:2023.2826
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https://doi.org/10.3390/pr10030599
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Feb 21, 2023
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